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2025-06-18
12:35

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2025-06-13
09:36
[IMPULSE-2025-00088] Journal Article
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Impact of local structure on melt dynamics in Cu-Ti alloys: Insights from ab initio molecular dynamics simulations
First-principles based molecular-dynamics simulations have been performed for binary Cu𝑥⁢Ti1−𝑥 (𝑥 = 0.31, 0.50, and 0.76) alloys to investigate the relationship between local structure and dynamical properties in the liquid and undercooled melt. The undercooled melts show a pronounced short-range order, majorly a fivefold symmetry (FFS) around the Cu atoms, which competes with bcc ordering. [...]
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2025-06-13
09:32
DBCoverage [IMPULSE-2025-00087] Journal Article
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Solvation Dynamics of Thermoresponsive Polymer Films: The Influence of Salt Series in Water and Mixed Water/Methanol Atmosphere
Advanced science 12(8), 2408073 () [10.1002/advs.202408073]
Understanding the salt effects on solvation behaviors of thermoresponsive polymers is crucial for designing and optimizing responsive systems suitable for diverse environments. In this work, the effect of potassium salts (CH 3 COOK, KCl, KBr, KI, and KNO3 ) on solvation dynamics of poly(4-(N- (3’-methacrylamidopropyl)-N,N-dimethylammonio) butane-1-sulfonate) (PSBP), poly(N-isopropylmethacrylamide) (PNIPMAM), and PSBP-b- PNIPMAM films is investigated under saturated water and mixed water/methanol vapor via advanced in situ neutron/optical characterization techniques. [...]
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2025-05-30
15:18
[IMPULSE-2025-00086] Journal Article
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Macroscopic and Microscopic Residual Stresses in Nickel-Aluminum Bronze Matrix Composite Surface Deposits Manufactured via Laser Melt Injection
Wear is a prevalent issue across various industries. Spherical fused tungsten carbide (sFTC) reinforced nickel-aluminum bronze (NAB) matrix composite surface deposits have shown remarkable potential in mitigating wear by approximately 80%. [...]
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2025-05-30
15:12
[IMPULSE-2025-00085] Journal Article
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Influence of current tabs on performance and aging of multi-tab 26650-type LFP lithium-ion batteries
Two high-power lithium-ion batteries of 26650-type adopting LiFePO4|C cell chemistry are non-invasively characterized using electrochemical, thermodynamical, and diffraction-based methods. Their discharging and charging behavior are probed using incremental capacity analysis and differential voltage analysis normalized to the state-of-charge. [...]
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2025-05-14
18:47
DBCoverage [IMPULSE-2025-00083] Journal Article
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Characterization of a mock up nuclear waste package using energy resolved MeV neutron analysis
Reliable radiographic methods for characterizing nuclear waste packages non-destructively (without the need to open containers) have the potential to significantly contribute to safe handling and future disposal options, particularly for legacy waste of unknown content. Due to required shielding of waste containers and the need to characterize materials consisting of light elements, X-ray methods are not suitable. [...]
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2025-05-14
18:26
[IMPULSE-2025-00082] Journal Article
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Exploring spatial resolution enhancements on IMAT for steel corrosion studies
Neutron imaging offers benefits over X-rays for steel corrosion studies including deep penetration and high sensitivity to some light elements such as hydrogen. However, the resolution is frequently at or below the thickness of the corroded layer. [...]
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2025-05-07
15:11
[IMPULSE-2025-00081] Journal Article
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Understanding the Role of Hydrogen and Oxygen in Electronic Phase Changes of Nickelates
Many electronic and electrochemical devices rely on the exchange of light elements such as hydrogen and oxygen with the environment. Understanding and tailoring the device functionality requires accurate information about the concentration and chemical bonding of such species inside a solid, which is particularly difficult if several species are exchanged. [...]
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2025-05-02
14:01
DBCoverage [IMPULSE-2025-00080] Journal Article
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Lattice-driven gating in a Cu-based zeolitic imidazolate framework for efficient high-temperature hydrogen isotope separation
For the separation of hydrogen isotopes (H2/D2), traditional kinetic quantum sieving (KQS) takes advantage of the diffusion barriers created by the flexibility of organic linkers and the breathing frameworks in porous solids. While the phenomena have been observed typically below 77 K, in this study, we present that a copper-based zeolite imidazolate framework (Cu-ZIF-gis) can show KQS above 120 K. [...]
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2025-05-02
13:59
[IMPULSE-2025-00079] Journal Article
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Soft phonon and the central peak at the cubic-to-tetragonal phase transition in SrTiO$_{3}$
The continuous displacive phase transition in SrTiO3 near 𝑇𝑐≈105 K features a central elastic peak in neutron-scattering investigations at temperatures above 𝑇𝑐, i.e., before the corresponding soft phonon mode is overdamped upon cooling. The origin of this central peak is still not understood. [...]
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